Phenothiazine Semiconducting Polymer for Light-Emitting Diodes
Identifieur interne : 000744 ( Main/Repository ); précédent : 000743; suivant : 000745Phenothiazine Semiconducting Polymer for Light-Emitting Diodes
Auteurs : RBID : Pascal:13-0158084Descripteurs français
- Pascal (Inist)
- Thiophène dérivé copolymère, Copolymère alterné, Copolymère hétérocyclique azote, Copolymère conjugué, Copolymère aromatique, Préparation, Polycondensation solution, Copulation Stille, Dérivé de la phénothiazine, Propriété électrochimique, Absorption optique, Diode électroluminescente organique, Courant court circuit, Brillance, Etude expérimentale, Phénothiazine dérivé copolymère, Benzodithiophène dérivé copolymère.
English descriptors
- KwdEn :
- Alternating copolymer, Aromatic copolymer, Brightness, Conjugated copolymer, Electrochemical properties, Experimental study, Nitrogen heterocycle copolymer, Optical absorption, Organic light emitting diodes, Phenothiazine derivatives, Preparation, Short circuit currents, Solution polycondensation, Stille coupling, Thiophene derivative copolymer.
Abstract
Phenothiazine alternating copolymer poly{4,8-bis(5-dodecylthiophene-2-yl)benzo[1,2-b:4,5-b'] dithiophene-alt-(10-decylphenothiazine)} (P1) is synthesized by Stille coupling polymerization. The synthesized polymer has an electrochemical bandgap of 1.61 eV and displays good photoluminescence with a quantum yield of 63.3%. The polymer is tested as a light-emitting material in polymeric light-emitting diodes (PLEDs) with a device structure of indium tin oxide (ITO)/poly(3,4-ethylenedioxythiophene) poly(styrenesulfonate) (PEDOT:PSS)/polymer/ Cs2CO3/Al. The devices display an orange-yellow electroluminescence (Commission Internationale de l'Eclairage (CIE) 1931 color-space chromaticity diagram: x = 0.5355 and y = 0.4611) with a maximum brightness of 3130 cd m-2 at an applied voltage of 10 V.
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<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Phenothiazine Semiconducting Polymer for Light-Emitting Diodes</title><author><name sortKey="Elkassih, Sussana A" uniqKey="Elkassih S">Sussana A. Elkassih</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Chemistry, University of Texas at Dallas, 800 West Campbell Road</s1><s2>Richardson, TX 75080</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>6 aut.</sZ><sZ>7 aut.</sZ></inist:fA14><country>États-Unis</country><wicri:noRegion>Richardson, TX 75080</wicri:noRegion></affiliation></author><author><name sortKey="Sista, Prakash" uniqKey="Sista P">Prakash Sista</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Chemistry, University of Texas at Dallas, 800 West Campbell Road</s1><s2>Richardson, TX 75080</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>6 aut.</sZ><sZ>7 aut.</sZ></inist:fA14><country>États-Unis</country><wicri:noRegion>Richardson, TX 75080</wicri:noRegion></affiliation></author><author><name sortKey="Magurudeniya, Harsha D" uniqKey="Magurudeniya H">Harsha D. Magurudeniya</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Chemistry, University of Texas at Dallas, 800 West Campbell Road</s1><s2>Richardson, TX 75080</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>6 aut.</sZ><sZ>7 aut.</sZ></inist:fA14><country>États-Unis</country><wicri:noRegion>Richardson, TX 75080</wicri:noRegion></affiliation></author><author><name sortKey="Papadimitratos, Alexios" uniqKey="Papadimitratos A">Alexios Papadimitratos</name><affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Solarno, Inc. 153 Hollywood Drive Coppell</s1><s2>TX 75019</s2><s3>USA</s3><sZ>4 aut.</sZ></inist:fA14><country>États-Unis</country><placeName><region type="state">Texas</region></placeName></affiliation></author><author><name sortKey="Zakhidov, Anvar A" uniqKey="Zakhidov A">Anvar A. Zakhidov</name><affiliation wicri:level="1"><inist:fA14 i1="03"><s1>Nanotech Institute, University of Texas at Dallas, 800 West Campbell Road</s1><s2>Richardson, TX 75080</s2><s3>USA</s3><sZ>5 aut.</sZ></inist:fA14><country>États-Unis</country><wicri:noRegion>Richardson, TX 75080</wicri:noRegion></affiliation></author><author><name sortKey="Biewer, Michael C" uniqKey="Biewer M">Michael C. Biewer</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Chemistry, University of Texas at Dallas, 800 West Campbell Road</s1><s2>Richardson, TX 75080</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>6 aut.</sZ><sZ>7 aut.</sZ></inist:fA14><country>États-Unis</country><wicri:noRegion>Richardson, TX 75080</wicri:noRegion></affiliation></author><author><name sortKey="Stefan, Mihaela C" uniqKey="Stefan M">Mihaela C. Stefan</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Chemistry, University of Texas at Dallas, 800 West Campbell Road</s1><s2>Richardson, TX 75080</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>6 aut.</sZ><sZ>7 aut.</sZ></inist:fA14><country>États-Unis</country><wicri:noRegion>Richardson, TX 75080</wicri:noRegion></affiliation></author></titleStmt><publicationStmt><idno type="inist">13-0158084</idno><date when="2013">2013</date><idno type="stanalyst">PASCAL 13-0158084 INIST</idno><idno type="RBID">Pascal:13-0158084</idno><idno type="wicri:Area/Main/Corpus">000F40</idno><idno type="wicri:Area/Main/Repository">000744</idno></publicationStmt><seriesStmt><idno type="ISSN">1022-1352</idno><title level="j" type="abbreviated">Macromol. chem. phys. : (Print)</title><title level="j" type="main">Macromolecular chemistry and physics : (Print)</title></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Alternating copolymer</term><term>Aromatic copolymer</term><term>Brightness</term><term>Conjugated copolymer</term><term>Electrochemical properties</term><term>Experimental study</term><term>Nitrogen heterocycle copolymer</term><term>Optical absorption</term><term>Organic light emitting diodes</term><term>Phenothiazine derivatives</term><term>Preparation</term><term>Short circuit currents</term><term>Solution polycondensation</term><term>Stille coupling</term><term>Thiophene derivative copolymer</term></keywords><keywords scheme="Pascal" xml:lang="fr"><term>Thiophène dérivé copolymère</term><term>Copolymère alterné</term><term>Copolymère hétérocyclique azote</term><term>Copolymère conjugué</term><term>Copolymère aromatique</term><term>Préparation</term><term>Polycondensation solution</term><term>Copulation Stille</term><term>Dérivé de la phénothiazine</term><term>Propriété électrochimique</term><term>Absorption optique</term><term>Diode électroluminescente organique</term><term>Courant court circuit</term><term>Brillance</term><term>Etude expérimentale</term><term>Phénothiazine dérivé copolymère</term><term>Benzodithiophène dérivé copolymère</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Phenothiazine alternating copolymer poly{4,8-bis(5-dodecylthiophene-2-yl)benzo[1,2-b:4,5-b'] dithiophene-alt-(10-decylphenothiazine)} (P1) is synthesized by Stille coupling polymerization. The synthesized polymer has an electrochemical bandgap of 1.61 eV and displays good photoluminescence with a quantum yield of 63.3%. The polymer is tested as a light-emitting material in polymeric light-emitting diodes (PLEDs) with a device structure of indium tin oxide (ITO)/poly(3,4-ethylenedioxythiophene) poly(styrenesulfonate) (PEDOT:PSS)/polymer/ Cs<sub>2</sub>CO<sub>3</sub>/Al. The devices display an orange-yellow electroluminescence (Commission Internationale de l'Eclairage (CIE) 1931 color-space chromaticity diagram: x = 0.5355 and y = 0.4611) with a maximum brightness of 3130 cd m<sup>-2</sup> at an applied voltage of 10 V.</div></front></TEI><inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>1022-1352</s0></fA01><fA03 i2="1"><s0>Macromol. chem. phys. : (Print)</s0></fA03><fA05><s2>214</s2></fA05><fA06><s2>5</s2></fA06><fA08 i1="01" i2="1" l="ENG"><s1>Phenothiazine Semiconducting Polymer for Light-Emitting Diodes</s1></fA08><fA11 i1="01" i2="1"><s1>ELKASSIH (Sussana A.)</s1></fA11><fA11 i1="02" i2="1"><s1>SISTA (Prakash)</s1></fA11><fA11 i1="03" i2="1"><s1>MAGURUDENIYA (Harsha D.)</s1></fA11><fA11 i1="04" i2="1"><s1>PAPADIMITRATOS (Alexios)</s1></fA11><fA11 i1="05" i2="1"><s1>ZAKHIDOV (Anvar A.)</s1></fA11><fA11 i1="06" i2="1"><s1>BIEWER (Michael C.)</s1></fA11><fA11 i1="07" i2="1"><s1>STEFAN (Mihaela C.)</s1></fA11><fA14 i1="01"><s1>Department of Chemistry, University of Texas at Dallas, 800 West Campbell Road</s1><s2>Richardson, TX 75080</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>6 aut.</sZ><sZ>7 aut.</sZ></fA14><fA14 i1="02"><s1>Solarno, Inc. 153 Hollywood Drive Coppell</s1><s2>TX 75019</s2><s3>USA</s3><sZ>4 aut.</sZ></fA14><fA14 i1="03"><s1>Nanotech Institute, University of Texas at Dallas, 800 West Campbell Road</s1><s2>Richardson, TX 75080</s2><s3>USA</s3><sZ>5 aut.</sZ></fA14><fA20><s1>572-577</s1></fA20><fA21><s1>2013</s1></fA21><fA23 i1="01"><s0>ENG</s0></fA23><fA43 i1="01"><s1>INIST</s1><s2>4111</s2><s5>354000503731420060</s5></fA43><fA44><s0>0000</s0><s1>© 2013 INIST-CNRS. All rights reserved.</s1></fA44><fA45><s0>33 ref.</s0></fA45><fA47 i1="01" i2="1"><s0>13-0158084</s0></fA47><fA60><s1>P</s1></fA60><fA61><s0>A</s0></fA61><fA64 i1="01" i2="1"><s0>Macromolecular chemistry and physics : (Print)</s0></fA64><fA66 i1="01"><s0>DEU</s0></fA66><fC01 i1="01" l="ENG"><s0>Phenothiazine alternating copolymer poly{4,8-bis(5-dodecylthiophene-2-yl)benzo[1,2-b:4,5-b'] dithiophene-alt-(10-decylphenothiazine)} (P1) is synthesized by Stille coupling polymerization. The synthesized polymer has an electrochemical bandgap of 1.61 eV and displays good photoluminescence with a quantum yield of 63.3%. The polymer is tested as a light-emitting material in polymeric light-emitting diodes (PLEDs) with a device structure of indium tin oxide (ITO)/poly(3,4-ethylenedioxythiophene) poly(styrenesulfonate) (PEDOT:PSS)/polymer/ Cs<sub>2</sub>CO<sub>3</sub>/Al. The devices display an orange-yellow electroluminescence (Commission Internationale de l'Eclairage (CIE) 1931 color-space chromaticity diagram: x = 0.5355 and y = 0.4611) with a maximum brightness of 3130 cd m<sup>-2</sup> at an applied voltage of 10 V.</s0></fC01><fC02 i1="01" i2="X"><s0>001D09D02E</s0></fC02><fC02 i1="02" i2="X"><s0>001D03F15</s0></fC02><fC03 i1="01" i2="X" l="FRE"><s0>Thiophène dérivé copolymère</s0><s2>NK</s2><s5>01</s5></fC03><fC03 i1="01" i2="X" l="ENG"><s0>Thiophene derivative copolymer</s0><s2>NK</s2><s5>01</s5></fC03><fC03 i1="01" i2="X" l="SPA"><s0>Tiofeno derivado copolímero</s0><s2>NK</s2><s5>01</s5></fC03><fC03 i1="02" i2="X" l="FRE"><s0>Copolymère alterné</s0><s2>NK</s2><s5>02</s5></fC03><fC03 i1="02" i2="X" l="ENG"><s0>Alternating copolymer</s0><s2>NK</s2><s5>02</s5></fC03><fC03 i1="02" i2="X" l="SPA"><s0>Copolímero alternado</s0><s2>NK</s2><s5>02</s5></fC03><fC03 i1="03" i2="X" l="FRE"><s0>Copolymère hétérocyclique azote</s0><s2>NK</s2><s5>03</s5></fC03><fC03 i1="03" i2="X" l="ENG"><s0>Nitrogen heterocycle copolymer</s0><s2>NK</s2><s5>03</s5></fC03><fC03 i1="03" i2="X" l="SPA"><s0>Copolímero heterocíclico nitrógeno</s0><s2>NK</s2><s5>03</s5></fC03><fC03 i1="04" i2="X" l="FRE"><s0>Copolymère conjugué</s0><s2>NK</s2><s5>05</s5></fC03><fC03 i1="04" i2="X" l="ENG"><s0>Conjugated copolymer</s0><s2>NK</s2><s5>05</s5></fC03><fC03 i1="04" i2="X" l="SPA"><s0>Copolímero conjugado</s0><s2>NK</s2><s5>05</s5></fC03><fC03 i1="05" i2="X" l="FRE"><s0>Copolymère aromatique</s0><s2>NK</s2><s5>06</s5></fC03><fC03 i1="05" i2="X" l="ENG"><s0>Aromatic copolymer</s0><s2>NK</s2><s5>06</s5></fC03><fC03 i1="05" i2="X" l="SPA"><s0>Copolímero aromático</s0><s2>NK</s2><s5>06</s5></fC03><fC03 i1="06" i2="X" l="FRE"><s0>Préparation</s0><s5>08</s5></fC03><fC03 i1="06" i2="X" l="ENG"><s0>Preparation</s0><s5>08</s5></fC03><fC03 i1="06" i2="X" l="SPA"><s0>Preparación</s0><s5>08</s5></fC03><fC03 i1="07" i2="X" l="FRE"><s0>Polycondensation solution</s0><s5>09</s5></fC03><fC03 i1="07" i2="X" l="ENG"><s0>Solution polycondensation</s0><s5>09</s5></fC03><fC03 i1="07" i2="X" l="SPA"><s0>Policondensación solución</s0><s5>09</s5></fC03><fC03 i1="08" i2="X" l="FRE"><s0>Copulation Stille</s0><s5>10</s5></fC03><fC03 i1="08" i2="X" l="ENG"><s0>Stille coupling</s0><s5>10</s5></fC03><fC03 i1="08" i2="X" l="SPA"><s0>Stille copulación</s0><s5>10</s5></fC03><fC03 i1="09" i2="X" l="FRE"><s0>Dérivé de la phénothiazine</s0><s1>ENT</s1><s5>12</s5></fC03><fC03 i1="09" i2="X" l="ENG"><s0>Phenothiazine derivatives</s0><s1>ENT</s1><s5>12</s5></fC03><fC03 i1="09" i2="X" l="SPA"><s0>Fenotiazina derivado</s0><s1>ENT</s1><s5>12</s5></fC03><fC03 i1="10" i2="X" l="FRE"><s0>Propriété électrochimique</s0><s5>13</s5></fC03><fC03 i1="10" i2="X" l="ENG"><s0>Electrochemical properties</s0><s5>13</s5></fC03><fC03 i1="10" i2="X" l="SPA"><s0>Propiedad electroquímica</s0><s5>13</s5></fC03><fC03 i1="11" i2="X" l="FRE"><s0>Absorption optique</s0><s5>15</s5></fC03><fC03 i1="11" i2="X" l="ENG"><s0>Optical absorption</s0><s5>15</s5></fC03><fC03 i1="11" i2="X" l="SPA"><s0>Absorción óptica</s0><s5>15</s5></fC03><fC03 i1="12" i2="3" l="FRE"><s0>Diode électroluminescente organique</s0><s5>16</s5></fC03><fC03 i1="12" i2="3" l="ENG"><s0>Organic light emitting diodes</s0><s5>16</s5></fC03><fC03 i1="13" i2="3" l="FRE"><s0>Courant court circuit</s0><s5>17</s5></fC03><fC03 i1="13" i2="3" l="ENG"><s0>Short circuit currents</s0><s5>17</s5></fC03><fC03 i1="14" i2="X" l="FRE"><s0>Brillance</s0><s5>19</s5></fC03><fC03 i1="14" i2="X" l="ENG"><s0>Brightness</s0><s5>19</s5></fC03><fC03 i1="14" i2="X" l="SPA"><s0>Brillantez</s0><s5>19</s5></fC03><fC03 i1="15" i2="X" l="FRE"><s0>Etude expérimentale</s0><s5>21</s5></fC03><fC03 i1="15" i2="X" l="ENG"><s0>Experimental study</s0><s5>21</s5></fC03><fC03 i1="15" i2="X" l="SPA"><s0>Estudio experimental</s0><s5>21</s5></fC03><fC03 i1="16" i2="X" l="FRE"><s0>Phénothiazine dérivé copolymère</s0><s2>NK</s2><s4>INC</s4><s5>32</s5></fC03><fC03 i1="17" i2="X" l="FRE"><s0>Benzodithiophène dérivé copolymère</s0><s2>NK</s2><s4>INC</s4><s5>33</s5></fC03><fC07 i1="01" i2="X" l="FRE"><s0>Propriété optique</s0><s5>14</s5></fC07><fC07 i1="01" i2="X" l="ENG"><s0>Optical properties</s0><s5>14</s5></fC07><fC07 i1="01" i2="X" l="SPA"><s0>Propiedad óptica</s0><s5>14</s5></fC07><fN21><s1>140</s1></fN21><fN44 i1="01"><s1>PSI</s1></fN44><fN82><s1>PSI</s1></fN82></pA></standard></inist></record>Pour manipuler ce document sous Unix (Dilib)
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